Don't forget to look behind you, as well. As the sun is setting below the horizon, it will throw some fantastic light onto the subjects behind you. So while you're waiting for that moment just after the sun disappears, turn around and check out the scenary behind you. Even a grungy city can have a beauty of it's own in the surreal glow of a fading sun...
But I will also say that investing in a graduated ND filter or three will help...a lot...
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